ErRe 3 is a rare example of a lanthanide single-molecule magnet coordinated solely by transition metals which enables the formulation of a promising strategy towards molecular intermetallic
Read MoreAbstract: The nanostructuring of single-molecule mag-nets (SMMs) on substrates, in nanotubes and periodic frameworks is highly desired for the future magnetic recording
Read MoreMagnetic materials are used to store digital information, and the magnetisation direction dictates if the storage bit is a 0 or a 1. The most important property for these materials is a bistable
Read MoreRare-earth based single-molecule magnets are promising candidates for magnetic information storage including qubits as their large magnetic moments are carried by localized 4f electrons. This shielding from the environment in turn hampers a direct electronic access to the magnetic moment. Here, we present the indirect readout of the
Read Moreingle-molecule magnets (SMMs) have been extensively investigated over the past two decades for their potential applications in the field of high-density data storage, molecular spintronics, and quantum calculation.[1] Unlike traditional ferromagnetic materials, the magnetism of SMMs is derived from the magnetic moment of a single molecule,[2]
Read MoreSingle molecule magnets (SMMs) constitute a pivotal class of nanoscale molecular magnets with promising potential across various domains such as high
Read MoreIn comparison, the previous record for a single-molecule magnet was 7.9 T at 10 K. The dysprosium complex also remained strongly magnetic at a relatively balmy 80 K, matching the highest recorded
Read Morea | Schematic representation of the energy diagram for a single-molecule magnet with S = 10 with energy equal to DS 2, where S is the spin state and D is the zero-field splitting parameter. The
Read MoreHere, we report the facile synthesis of two discrete highly thermally stable lanthanide compounds, Ln (hfac) 3 (TPE-tz) (Ln=Eu, Dy), by the reaction of the AIE-active organic ligand with Ln (III) β-diketonate precursor. Due to different energy gaps between the triplet state of the ligand and the accepted level of Ln (III) ions, Eu (hfac) 3
Read MoreMagnets formed from a single molecule are of particular interest in data storage, since the ability to store a bit on every molecule could vastly increase the storage capacity of computers.
Read MoreThe observation of a magnetic memory effect 3 in single-molecule magnets (SMMs) has represented a breakthrough in nanomagnetism 10 has opened the exciting perspective of exploiting the
Read MoreRare-earth based single-molecule magnets are promising candidates for magnetic information storage including qubits as their large magnetic moments are
Read MoreUnique Double and Triple Decker Arrangements of Rare-Earth 9,10-Diborataanthracene Complexes Featuring Single-Molecule Magnet Characteristics. Cedric -earth ions in 3-Ln, whereas in the presence of a potassium ion in 2-Ln, more electron density is transferred to one single rare-earth ion. A similar energy diagram is
Read More1. Introduction Molecular-based magnetic materials draw a lot of attention due to their potential applications in high-density information storage, 1, 2, 3 low-temperature magnetic refrigeration 4, 5 and spin-based qubits for quantum computing. 6, 7 In these applications the inherent magnetic anisotropy of molecular magnetic materials
Read MoreScientific Reports (2021) Molecular magnets are promising for their use as high-density memory devices. However, maintaining the molecules'' magnetic state when bonded to a substrate has been
Read MoreMolecular design and device fabrication. With these principles in mind, we designed the molecule MP (Fig. 2a), which consists of a trivalent rare-earth ion (M), coordinated by a redox-active
Read MoreIntroduction. Lanthanide-based single molecule magnets (SMMs) are a fascinating class of coordination compounds built by Ln 3+ ions coordinated to organic or inorganic ligands, which exhibit a slow relaxation of the magnetization and a magnetic hysteresis at the molecular level. Unlike traditional bulk magnets composed of a large
Read MoreSingle-molecule magnets (SMMs) offer stable quantum objects capable of exhibiting diverse magnetic states on the nanoscale, making them promising candidates for storing and processing quantized information at the molecular level. While substantial
Read MoreMany of the most industrially important magnets require the addition of rare-earths to improve their coercivity and magnetic performance. Here, the authors place a single paramagnetic rare-earth
Read MoreAbstract. Molecular toolkit is a crucial part of futuristic spintronics and quantum information technologies. Magnetic bistability is the basis for such applications,
Read MoreMagnetic studies indicated that, despite the low C 2 symmetry, 1 and 2 display single molecule magnet (SMM) behavior, with 1 exhibiting an effective energy barrier of the relaxation of the magnetization U eff /k B = 50 K and the pre-exponential factor τ o = 6.80 × 10 –7 s. Step-like features in the hysteresis loops indicate the presence of
Read MoreSingle-Molecule Magnets Unique Double and Triple Decker Arrangements of Rare-Earth 9,10-Diborataanthracene Complexes Featuring Single-Molecule Magnet Characteristics Cedric Uhlmann, Luca Münzfeld, Adrian Hauser, Ting-Ting Ruan, Senthil Kumar Kuppusamy, Chengyu Jin, Mario Ruben, Karin Fink, Eufemio Moreno-Pineda,* and Peter
Read MoreRare-earth based single-molecule magnets are promising candidates for magnetic information storage including qubits as their large magnetic moments are carried by localized 4 f electrons. This shielding from the environment in turn hampers a direct electronic access to the magnetic moment. Here, we present the indirect readout of the
Read MoreThe aim was then to design single-molecule magnets (SMMs) exhibiting memory effects at higher temperatures. This difference explains why the energy barriers of SIMs based on rare-earth ions
Read MoreWe discuss a cost-effective approach to understand magnetic relaxation in the new generation of rare-earth single-molecule magnets. It combines ab initio calculations of the crystal field parameters, of the magneto-elastic
Read MoreIn this review, the recent progress in rare earth SMMs represented by mononuclear and dinuclear complexes is highlighted, especially for the modulation of
Read MoreHere, we report the incorporation of magnetic (RECl 2 (H 2 O) 6) + (RE=rare earths) molecular groups into the framework of an organic metal halide
Read MoreRare earth SMMs are considered to be the most promis-ing for application owing to their large magnetic moment and strong magnetic anisotropy. In this review, the recent progress in rare earth SMMs represented by mononuclear and dinuclear com-plexes is highlighted, especially for the modulation of magnetic anisotropy, effective
Read MoreResearchers have now developed a new molecular system with a particular magnetic hardness. The ingredients in this special recipe are rare earth metals and an unusual nitrogen-based molecular
Read MoreMission Statement. The goal of the Eddleman Quantum Institute at UCI is to stimulate the discovery of new quantum science phenomena by developing collaborations between investigators in a broad range of scientific endeavors and to motivate future generations to study quantum science through educational and outreach activities.
Read MoreThe demonstration of magnetic bistability in single-molecule magnets containing one rare-earth atom 4,6,9,11 illustrated the potential of single-atom spin centres in future storage media 5,7,8,10
Read MoreThis FE SMM also shows single-molecule magnetic behaviors, toroidal magnetic moments, and room-temperature ferroelectricity. The toroidal moment is formed by a vortex distribution of magnetic dipoles in triangular Dy 3 clusters. The analysis of ac magnetic susceptibility reveals the coexistence of three distinct magnetic relaxation processes at
Read MoreQuench calculations were used to obtain the energy minima for a single Mn 12 (acetate) 16 molecule on the Au(111) surface. In these quench calculations, an MD simulation is performed, and at
Read MoreStudies of RE-POM single-molecule magnets (SMMs) have utilized magnetic susceptibility, inelastic neutron scattering, and ab initio calculations. These investigations have allowed characterization of the crystal field splitting of the rare earth(III) ions that is responsible for the SMM properties of slow magnetic relaxation and
Read MoreMagnetic molecules known as molecular nanomagnets (MNMs) may be the key to ultra-high density data storage. Thus, novel strategies on how to design MNMs are desirable.
Read MoreHere, we report the incorporation of magnetic (RECl 2 (H 2 O) 6) + (RE=rare earths) molecular groups into the framework of an organic metal halide perovskite (OMHP)-(H 2 dabco)CsCl 3. Intriguingly, we show the incorporated rare-earth groups self-organized into long-range ordered arrays that uniformly and periodically distributed in the
Read MoreIn general, a magnetic molecule is a metal–organic complex bearing a stable net spin moment, which originates from a single magnetic ion, a transition metal or a rare earth, or from a collection
Read MoreThis FE SMM also shows single‐molecule magnetic behaviors, toroidal magnetic moments, and room‐temperature ferroelectricity. The toroidal moment is formed by a vortex distribution of magnetic dipoles in triangular Dy 3 clusters. The analysis of ac magnetic susceptibility reveals the coexistence of three distinct magnetic relaxation
Read MoreSingle molecule magnets (SMMs) constitute a pivotal class of nanoscale molecular magnets with promising potential across various domains such as high-density information storage, quantum computing, and spin electron devices. Among these, lanthanide-based SMMs have garnered significant attention in recent research due to
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